Department of Chemical and Metallurgical Engineering

Metallurgy

The Research Group for Metallurgy is led by Prof. Ari Jokilaakso, and our activities cover a large area from the life span of a metal product, starting from the making of metal, continuing with the making of metal products and their behaviour at high temperatures and ending in recycling and waste utilisation.
Pyrometallurgy_research Ronja Ruismäki, photo Valeria Azovskaya

Our research areas:

  1. Physicochemical fundamentals and modelling of metallurgical operations

  2. Kinetics of metallurgical reactions especially in non-ferrous metals production

  3. Recycling of e-scrap and energy storage materials in pyrometallurgical processes

The current research activities focus on physicochemical fundamentals and modelling of metallurgical operations, slags, mattes, ceramics and other high-temperature materials. Processes that benefit from this research include modern extractive and refining processes for ferrous and non-ferrous metals, casting and solidification as well as materials synthesis and behaviour at high temperatures. The main emphasis is on better understanding of metallurgical phenomena by combining experimental studies with computer simulation and modelling.

The Group’s strengths include expertise in thermodynamics, kinetics and transport phenomena as well as solid qualification in experimental research and material characterization.

Our research highlights:

Beheviour of batteries
A typical sample microstructure
  • Behavior of Battery Metals Lithium, Cobalt, Manganese and Lanthanum in Black Copper Smelting:

Recycling of metals from different waste streams must be increased in the near future for securing the availability of metals that are critical for high-tech applications, such as batteries for e-mobility. Black copper smelting is a flexible recycling route for many different types of scrap, including Waste Electrical and Electronic Equipment (WEEE) and some end-of-life energy storage materials. Fundamental thermodynamic data about the behavior of battery metals and the effect of slag additives is required for providing data necessary for process development, control, and optimization. The goal of our study is to investigate the suitability of black copper smelting process for recycling of battery metals lithium, cobalt, manganese, and lanthanum.

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Outotec flash smelting furnace
Illustration of the Outotec flash smelting furnace
  • Computational Approaches for Studying Slag–MatteInteractions in the Flash Smelting Furnace(FSF) Settler:

Computational methods have become reliable tools in many disciplines for research andindustrial design. There are, however, an ever-increasing number of details waiting to be included in the models and software, including, e.g., chemical reactions and many physical phenomena, such asparticle and droplet behavior and their interactions. The dominant method for copper production,flash smelting, has been extensively investigated, but the settler part of the furnace containing moltenhigh temperature melts termed slag and matte, still lacks a computational modeling tool. In this paper,two commercial modeling software programs have been used for simulating slag–matte interactionsin the settler, the target being first to develop a robust computational fluid dynamics (CFD) modeland, second, to apply a new approach for molten droplet behavior in a continuum. The latter isbased on CFD coupled with the discrete element method (DEM), which was originally developedfor modeling solid particle–particle interactions and movement, and is applied here for individualdroplets for the first time.

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Kinetics_rare elements
A): SEM-secondary electron image of laser pits in matte phase. (B): Time-resolved analysis signals for neodymium (143Nd) of the LA-ICP-MS measurements on the copper sulfide mattes of samples contacted in air for 20 s and 300 s at 1300 °C.
  • Distribution Kinetics of Rare Earth Elements in Copper Smelting:

The use of rare earth elements (REEs) is increasing, mainly due to the growing demand for electric vehicles and new applications in green technology. This results in annual growth of the in-use REE stocks and the amount of End-of-Life (EoL) products containing REEs. REEs are considered critical elements by the EU, mainly because the rest of the world is dependent on China’s supply. Recycling of REEs can help alleviate the criticality of REEs, however, no REEs are currently functionally recycled. In this study, the time-dependent behavior of REEs in copper matte-slag system in primary copper smelting conditions was investigated experimentally at a laboratory scale.

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LabPhoto_Glen Forde

“Metallurgy – Work that has a meaning”: metallurgy / metallurgists will save the world as the modern life is not possible without metals.

Ari Jokilaakso

"Green” energy and electrification of vehicles need more metals (exponentially increasing amounts) and, therefore, metals production has to be developed for maximized yield and all metal products should be recycled back to metals production, which necessitates metallurgical basic research work.

- Ari Jokilaakso

Related content:

Professor Ari Jokilaakso visited A-Studio on Monday, 15th March 2021 (external link)

The topic was about cobalt coming from the Republic of the Congo and the ethical challenges related to it. This clip starts at min. 23.25 (In Finnish).

Ari Jokilaakso, A-studio

Towards carbon-neutrality in metal production – new €18 million project to develop solutions for reducing CO2 emissions

Metal processing industry has the greatest greenhouse gas reduction potential of Finland's manufacturing industries. Joint project between companies and universities is a significant step towards carbon-neutral metal production.

Metalls, CMET

Invitation to SYMMET results webinar on 26.11.2020

The production from current mines is not sufficient to fulfil the need for metals, especially when clean
energy, e.g. wind and solar, and electric vehicles are produced in growing amounts. SYMMET is trying
to find answers to the sustainability gap, which is the result of continuously increasing need for
metallic materials.

Yhteistyökumppanit

How to get companies in the metal industry more employees and more students for the master’s degree programme?

‘The great thing about this cooperation is that everyone wins,’ said Ari Jokilaakso, Professor of metallurgy.

Department of Chemistry and Materials Science

The sustainable use of metals is at the core of fighting climate change – It’s no use to substitute walking with electric scooters

Electric cars and electric scooters are not environmentally friendly options if they are used as an alternative to walking or cycling, for example. Different metals are constantly needed in increasing amounts for batteries, for example. The challenge is both ecological and social.

akkumetalli kierrätys batchircle

Half a million funding from Business Finland for the development of circular economy of metals

The funded sub-project of Aalto is part of SYMMET, which is searching for solutions to the increasing need for metallic materials.

Metallurgian tutkimuslaitteistoa / kuva: Glen Forde

Metallurgists are needed to fix the sustainability gap

Professor of Metallurgy Ari Jokilaakso’s researches the behaviour of chemical elements at high temperatures. He wants to give students a real understanding of chemical phenomena.

Photo: Mikko Raskinen

Metals needed for climate solutions – will what we have be enough?

Metal recovery and production processes using secondary raw materials must be developed and awareness of the need for recycling increased.

Liikenne / kuva: Adolfo Vera

Latest publications:

Solubility of Palladium in Alumina-Iron Silicate Melts

Katri Avarmaa, Lassi Klemettinen, Hugh O’Brien, Ari Jokilaakso, Daniel Lindberg, Pekka Taskinen 2021 JOM

Precious Metal Distributions Between Copper Matte and Slag at High PSO2 in WEEE Reprocessing

Min Chen, Katri Avarmaa, Lassi Klemettinen, Hugh O’Brien, Junjie Shi, Pekka Taskinen, Daniel Lindberg, Ari Jokilaakso 2021 Metallurgical and Materials Transactions B: Process Metallurgy and Materials Processing Science

Treatment of high-arsenic copper smelting flue dust with high copper sulfate : Arsenic separation by low temperature roasting

Yujie Chen, Shun Zhu, Pekka Taskinen, Ning Peng, Bing Peng, Ari Jokilaakso, Hui Liu, Yanjie Liang, Zongwen Zhao, Zhongbing Wang 2021 Minerals Engineering

The efficiency of scrap Cu and Al current collector materials as reductants in LIB waste leaching

Alexander Chernyaev, Jere Partinen, Lassi Klemettinen, Benjamin P. Wilson, Ari Jokilaakso, Mari Lundström 2021 Hydrometallurgy

Worth from waste: Utilizing a graphite‐rich fraction from spent lithium‐ion batteries as alternative reductant in nickel slag cleaning

Anna Danczak, Ronja Ruismäki, Tommi Rinne, Lassi Klemettinen, Hugh O’Brien, Pekka Taskinen, Ari Jokilaakso, Rodrigo Serna‐Guerrero 2021 Minerals

Iron activity measurements and spinel-slag equilibria in alumina-bearing iron silicate slags

Lassi Klemettinen, Katri Avarmaa, Ari Jokilaakso, Pekka Taskinen 2021 Journal of Alloys and Compounds

Clean antimony production from stibnite concentrate with goethite residue co-treatment for zinc, iron, sulfur conservation

Yun Li, Haotian Xue, Pekka Taskinen, Ari Jokilaakso, Chaobo Tang, Wei Jin, Minna Rämä, Yongming Chen, Shenghai Yang 2021 Journal of Cleaner Production

PbSO4 Reduction Mechanism and Gas Composition at 600–1000°C

Yun Li, Pekka Taskinen, Yuejun Wang, Shenghai Yang, Chaobo Tang, Yongming Chen, Ari Jokilaakso 2021 JOM

Selective separation of rare earths from spent Nd-Fe-B magnets using two-stage ammonium sulfate roasting followed by water leaching

Fupeng Liu, Feixiong Chen, Longjun Wang, Shuaibing Ma, Xingbang Wan, Jinliang Wang 2021 Hydrometallurgy

Optimization of the CCT Curves for Steels Containing Al, Cu and B

Jyrki Miettinen, Sami Koskenniska, Mahesh Somani, Seppo Louhenkilpi, Aarne Pohjonen, Jari Larkiola, Jukka Kömi 2021 Metallurgical and Materials Transactions B: Process Metallurgy and Materials Processing Science
More information on our research in the Research database.
Research database
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